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enter image description here

As you can clearly see in the high quality diagram above, I'm looking for a way to get the nitrogen and hydrogen bonded like that in chemfig.

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You're looking for \chemabove{<atom>}{<above>}:

\documentclass{article}
\usepackage{chemfig}

\begin{document}

\chemfig{R^1-[:30]\chemabove{N}{H}-[:-30]R^2}

\end{document}

enter image description here

Just for the record: there's also \chembelow{<atom>}{<below>}. I've described them in a little more detail in my answer to “Changing space between atoms in Chemabove

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