NOTE: I have added a second example, where only one table uses the indented notes. Also in this example \linewidth
is used instead of \textwidth
.
\documentclass{article}
\usepackage{tabularray}
\begin{document}
\newlength\labellength
\DefTblrTemplate{remark}{default}{%
\MapTblrRemarks{%
\settowidth{\labellength}{\UseTblrTemplate{remark-tag}{default}\UseTblrTemplate{remark-sep}{default}}%
\UseTblrTemplate{remark-tag}{default}\UseTblrTemplate{remark-sep}{default}%
\parbox[t]{\dimexpr\textwidth-\labellength}{\UseTblrTemplate{remark-text}{default}}%
\par
}}
\begin{table}[htbp]
\begin{talltblr}[
caption={table},
remark{Hello}={It is a very long note.It is a very long note.It is a very long note.It is a very long note.It is a very long note.It is a very long note.}
]{
colspec={X[c] *{2}{X[c,2]}}
}
&HI&HI\\
low&$<10$&$<0$\\
me&$20\leq\quad\leq 30$&$40\leq\quad\leq 50$\\
hogh&$>0$&$>50$\\
\end{talltblr}
\end{table}
\end{document}

Second example: Here I use a theme, so that you can choose which tables use the solution.
\documentclass{article}
\usepackage{tabularray}
\begin{document}
\newlength\labellength
\DefTblrTemplate{remark}{indentednotes}{%
\MapTblrRemarks{%
\settowidth{\labellength}{\UseTblrTemplate{remark-tag}{default}\UseTblrTemplate{remark-sep}{default}}%
\UseTblrTemplate{remark-tag}{default}\UseTblrTemplate{remark-sep}{default}%
\parbox[t]{\dimexpr\linewidth-\labellength}{\UseTblrTemplate{remark-text}{default}}%
\par}
}
\NewTblrTheme{indentednotes}{
\SetTblrTemplate{remark}{indentednotes}
}
\begin{table}[htbp]
\begin{talltblr}[
theme = indentednotes,
caption={table with indented notes},
remark{Hello}={It is a very long note.It is a very long note.It is a very long note.It is a very long note.It is a very long note.It is a very long note.}
]{
colspec={X[c] *{2}{X[c,2]}}
}
&HI&HI\\
low&$<10$&$<0$\\
me&$20\leq\quad\leq 30$&$40\leq\quad\leq 50$\\
hogh&$>0$&$>50$\\
\end{talltblr}
\end{table}
\begin{table}[htbp]
\begin{talltblr}[
caption={table with normal notes},
remark{Hello}={It is a very long note.It is a very long note.It is a very long note.It is a very long note.It is a very long note.It is a very long note.}
]{
colspec={X[c] *{2}{X[c,2]}}
}
&HI&HI\\
low&$<10$&$<0$\\
me&$20\leq\quad\leq 30$&$40\leq\quad\leq 50$\\
hogh&$>0$&$>50$\\
\end{talltblr}
\end{table}
\end{document}